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University of Illinois at Urbana-Champaign

Dynamics of Dissociative Chemisorption: Methane on Tungsten Single Crystal Surfaces

Abstract

dc:description

Chemisorption of simple molecular gases on clean metal surfaces is usually rapid, with vanishingly small activation energies and large sticking coefficients. However, for more complicated molecules, such as saturated hydrocarbons, chemisorption is often a slow process which involves thermal excitation over relatively high barriers. We have studied one such system: the dissociation of methane on clean tungsten single crystal surfaces. The purpose of this study is to explore the nature of the elementary excitations which bring about dissociation and subsequent adsorption. Our effort has been concentrated upon studying the effect of thermal excitations of the gas as well as the importance of the crystal structure of the metal surface.

Degree

thesis:*
Name thesis:degree_name
Ph.D.
Level thesis:degree_level
Dissertation
Discipline thesis:degree_discipline
Physics
Grantor
University of Illinois at Urbana-Champaign
Year dc:date
2015

Author and committee

dc:creator, dc:contributor.*
Author dc:creator
  • Lo, Tai-Chin

Subjects

dc:subject × 1

Rights

Language dc:language
eng

Identifiers

dc:identifier.*
Identifier
(UMI)AAI8309976
OAI identifier oai:identifier
oai:www.ideals.illinois.edu:2142/77351

Chain of custody

source
Harvested from
University of Illinois - Urbana-Champaign
Base URL
www.ideals.illinois.edu/oai-pmh
Last updated
2026-07-22
Source record
OAI-PMH GetRecord
citation

Lo, Tai-Chin. Dynamics of Dissociative Chemisorption: Methane on Tungsten Single Crystal Surfaces. Dissertation thesis, University of Illinois at Urbana-Champaign, 2015. http://hdl.handle.net/2142/77351