Spatiotemporal variation of PM2.5 over the contiguous United States
type: CreativeWork
description: PM2.5 is the set of airborne particulate matter (also known as aerosols) with diameter 2.5 m or smaller. Ambient concentrations of these aerosols have been shown to be highly correlated with premature mortality throughout the world. Previous studies on ground-level, in-situ PM 2.5 concentrations have explored the diurnal and seasonal variation, but have been limited to small geographic areas. This research aims to identify the locations, times of day, and months of the year at which people are most likely to be exposed to high PM2.5 concentrations using data from ground monitors across the contiguous United States. K-means clustering was utilized to group of the diurnal and seasonal cycles by their shape in order to explore multi-scale temporal variations across the United States. Two distinct groups of diurnal cycles appeared in summer (June, July, August) and winter (December, January, February), with maxima occurring in the morning (0700 local time in the summer and 0800 in the winter) and the evening (roughly 20:00). Further, we found that the seasonal cycles are also separated into two clusters: one that has a summertime maximum, and the other with distinct winter and summer maxima. County-level spatial heterogeneity of PM2.5 was examined to quantify why monitors in similar areas may appear in different clusters. The correlation (Pearson's r) between monitors varies highly by county, which may be influenced by the placement of monitors with respect to emission sources of PM2.5. The correlation decreased with increasing distance between them, but that the correlation depended more strongly on the specific county in which the monitors are located. We quantified the covariation of PM2.5 with other pollutants to determine if we can separate their effects on human health for epidemiological studies. We found that PM2.5 is often positively correlated (r approximately equal to .5) with CO and NO2, with varying correlation when using different temporally averaged measu…
abstract: PM2.5 is the set of airborne particulate matter (also known as aerosols) with diameter 2.5 m or smaller. Ambient concentrations of these aerosols have been shown to be highly correlated with premature mortality throughout the world. Previous studies on ground-level, in-situ PM 2.5 concentrations have explored the diurnal and seasonal variation, but have been limited to small geographic areas. This research aims to identify the locations, times of day, and months of the year at which people are most likely to be exposed to high PM2.5 concentrations using data from ground monitors across the contiguous United States. K-means clustering was utilized to group of the diurnal and seasonal cycles by their shape in order to explore multi-scale temporal variations across the United States. Two distinct groups of diurnal cycles appeared in summer (June, July, August) and winter (December, January, February), with maxima occurring in the morning (0700 local time in the summer and 0800 in the winter) and the evening (roughly 20:00). Further, we found that the seasonal cycles are also separated into two clusters: one that has a summertime maximum, and the other with distinct winter and summer maxima. County-level spatial heterogeneity of PM2.5 was examined to quantify why monitors in similar areas may appear in different clusters. The correlation (Pearson's r) between monitors varies highly by county, which may be influenced by the placement of monitors with respect to emission sources of PM2.5. The correlation decreased with increasing distance between them, but that the correlation depended more strongly on the specific county in which the monitors are located. We quantified the covariation of PM2.5 with other pollutants to determine if we can separate their effects on human health for epidemiological studies. We found that PM2.5 is often positively correlated (r approximately equal to .5) with CO and NO2, with varying correlation when using different temporally averaged measu…
author: CrowleyFarenga, Remy Michael John
language: en
keywords: PM2.5, spaiotemporal, seasonal, diurnal, covariation, pollution, particulate matter, united states
date published: 2018-09-27T16:18:00Z
date modified: 2026-07-22T22:24:40Z
provider: University of Illinois - Urbana-Champaign
publisher: Networked Digital Library of Theses and Dissertations
type: WebPage
source organization: University of Illinois at Urbana-Champaign

PropertyValue
property ID: Handle
value: http://hdl.handle.net/2142/101621