{"id":{"repo_id":"cape-town","oai_identifier":"oai:open.uct.ac.za:11427/36466"},"canonical_url":"https://search.dev.ndltd.org/etd/cape-town/oai:open.uct.ac.za:11427/36466","repository":{"repo_id":"cape-town","name":"University of Cape Town","base_url":"https://open.uct.ac.za/oai/request"},"display":{"title":"Multi-photon decay mode spectroscopy of positronium","abstract":"An approximation for the branching ratio of the four-photon decay of parapositronium (BR4γ) was measured using a multi-gamma-ray spectrometer. For the first time in such measurements, the spectrometer consisted of an array of eight identical LaBr3:Ce scintillator detectors, each of which combines good energy resolutions (5% and 10% at 511 keV for the signals from the eighth dynode and anode of the photomultiplier tube, respectively) with an excellent timing resolution (∼ 300 ps). These energy resolutions were minimised through an optimal selection of the digital signal processing parameter settings. The detectors were situated in a planar geometry, where the source-to-detector distance of the detector system was selected such that the effect of peak pulse pile-up was minimised (to less than 3%), while maximising the full-energy peak detection efficiency at 511 keV (to 3%). For this work, locally-produced 22Na radioactive sources were used as positron emitters, which enabled the formation of positronium and subsequent gamma decays. Energy calibration measurements were performed using a 152Eu source, where the prominent energy peaks of (121.8, 244.7, 344.3, 778.9, 964.1, 1408.0) keV were used for calibration. For the BR4γ measurement, 5×1011 events were accumulated over a measurement period of 60 days, which resulted in low statistical uncertainties for the coincident counting between detector pairs (less than 1%). Through simplifying assumptions that neglected the background corrections and efficiency normalisations for each of the 2γ and 4γ decays, a first order approximation of BR4γ was determined as the ratio between measured 4γ events (N4γ) and measured 2γ events (N2γ), such that BR4γ ∼ N4γ N2γ = 4.8 (19) × 10−7. This measured value of BR4γ differs from previous measurements and accepted literature values by a factor of 3.","abstract_html":"An approximation for the branching ratio of the four-photon decay of parapositronium (BR4γ) was measured using a multi-gamma-ray spectrometer. For the first time in such measurements, the spectrometer consisted of an array of eight identical LaBr3:Ce scintillator detectors, each of which combines good energy resolutions (5% and 10% at 511 keV for the signals from the eighth dynode and anode of the photomultiplier tube, respectively) with an excellent timing resolution (∼ 300 ps). These energy resolutions were minimised through an optimal selection of the digital signal processing parameter settings. The detectors were situated in a planar geometry, where the source-to-detector distance of the detector system was selected such that the effect of peak pulse pile-up was minimised (to less than 3%), while maximising the full-energy peak detection efficiency at 511 keV (to 3%). For this work, locally-produced 22Na radioactive sources were used as positron emitters, which enabled the formation of positronium and subsequent gamma decays. Energy calibration measurements were performed using a 152Eu source, where the prominent energy peaks of (121.8, 244.7, 344.3, 778.9, 964.1, 1408.0) keV were used for calibration. For the BR4γ measurement, 5×1011 events were accumulated over a measurement period of 60 days, which resulted in low statistical uncertainties for the coincident counting between detector pairs (less than 1%). Through simplifying assumptions that neglected the background corrections and efficiency normalisations for each of the 2γ and 4γ decays, a first order approximation of BR4γ was determined as the ratio between measured 4γ events (N4γ) and measured 2γ events (N2γ), such that BR4γ ∼ N4γ N2γ = 4.8 (19) × 10−7. This measured value of BR4γ differs from previous measurements and accepted literature values by a factor of 3.","abstract_has_math":false,"creators":["Johnson, Storm"],"institution":"Department of Physics","degree_name":null,"degree_level":null,"degree_discipline":null,"degree_department":null,"school":null,"contributors":[],"advisors":["Leadbeater, Thomas","Jones, Pete"],"committee_chairs":[],"committee_members":[],"year":2022,"date_issued":"2022","date_published":"2022","updated_at":"2026-07-22T22:23:41Z","subjects":["Physics"],"languages":[],"rights":[],"rights_urls":[],"identifier_entries":[]},"links":{"outbound_url":"http://hdl.handle.net/11427/36466","outbound_label":"Handle","outbound_source":"dc:identifier.uri"},"metadata_groups":[{"id":"people","label":"People","entries":[{"key":"dc:contributor.advisor","label":"Advisor","values":["Leadbeater, Thomas","Jones, Pete"]},{"key":"dc:creator","label":"Author","values":["Johnson, Storm"]}]},{"id":"academic_context","label":"Academic Context","entries":[{"key":"dc:date.accessioned","label":"Dc Date Accessioned","values":["2022-06-10T10:11:07Z"]},{"key":"dc:date.available","label":"Dc Date Available","values":["2022-06-10T10:11:07Z"]},{"key":"dc:date.issued","label":"Date","values":["2022"]},{"key":"dc:publisher.department","label":"Dc Publisher Department","values":["Department of Physics"]},{"key":"dc:type","label":"Dc Type","values":["Master Thesis"]},{"key":"dc:type.qualificationlevel","label":"Dc Type Qualificationlevel","values":["Masters","MSc"]}]},{"id":"subjects_keywords","label":"Subjects and Keywords","entries":[{"key":"dc:subject","label":"Dc Subject","values":["Physics"]}]},{"id":"identifiers","label":"Identifiers","entries":[{"key":"dc:identifier.uri","label":"Identifier URI","values":["http://hdl.handle.net/11427/36466"]}]},{"id":"additional","label":"Additional Metadata","entries":[{"key":"dc:description.abstract","label":"Abstract","values":["An approximation for the branching ratio of the four-photon decay of parapositronium (BR4γ) was measured using a multi-gamma-ray spectrometer. For the first time in such measurements, the spectrometer consisted of an array of eight identical LaBr3:Ce scintillator detectors, each of which combines good energy resolutions (5% and 10% at 511 keV for the signals from the eighth dynode and anode of the photomultiplier tube, respectively) with an excellent timing resolution (∼ 300 ps). These energy resolutions were minimised through an optimal selection of the digital signal processing parameter settings. The detectors were situated in a planar geometry, where the source-to-detector distance of the detector system was selected such that the effect of peak pulse pile-up was minimised (to less than 3%), while maximising the full-energy peak detection efficiency at 511 keV (to 3%). For this work, locally-produced 22Na radioactive sources were used as positron emitters, which enabled the formation of positronium and subsequent gamma decays. Energy calibration measurements were performed using a 152Eu source, where the prominent energy peaks of (121.8, 244.7, 344.3, 778.9, 964.1, 1408.0) keV were used for calibration. For the BR4γ measurement, 5×1011 events were accumulated over a measurement period of 60 days, which resulted in low statistical uncertainties for the coincident counting between detector pairs (less than 1%). Through simplifying assumptions that neglected the background corrections and efficiency normalisations for each of the 2γ and 4γ decays, a first order approximation of BR4γ was determined as the ratio between measured 4γ events (N4γ) and measured 2γ events (N2γ), such that BR4γ ∼ N4γ N2γ = 4.8 (19) × 10−7. This measured value of BR4γ differs from previous measurements and accepted literature values by a factor of 3."]},{"key":"dc:title","label":"Title","values":["Multi-photon decay mode spectroscopy of positronium"]}]}],"canonical_facts":{"dc:contributor.advisor":["Leadbeater, Thomas","Jones, Pete"],"dc:creator":["Johnson, Storm"],"dc:date.accessioned":["2022-06-10T10:11:07Z"],"dc:date.available":["2022-06-10T10:11:07Z"],"dc:date.issued":["2022"],"dc:description.abstract":["An approximation for the branching ratio of the four-photon decay of parapositronium (BR4γ) was measured using a multi-gamma-ray spectrometer. For the first time in such measurements, the spectrometer consisted of an array of eight identical LaBr3:Ce scintillator detectors, each of which combines good energy resolutions (5% and 10% at 511 keV for the signals from the eighth dynode and anode of the photomultiplier tube, respectively) with an excellent timing resolution (∼ 300 ps). These energy resolutions were minimised through an optimal selection of the digital signal processing parameter settings. The detectors were situated in a planar geometry, where the source-to-detector distance of the detector system was selected such that the effect of peak pulse pile-up was minimised (to less than 3%), while maximising the full-energy peak detection efficiency at 511 keV (to 3%). For this work, locally-produced 22Na radioactive sources were used as positron emitters, which enabled the formation of positronium and subsequent gamma decays. Energy calibration measurements were performed using a 152Eu source, where the prominent energy peaks of (121.8, 244.7, 344.3, 778.9, 964.1, 1408.0) keV were used for calibration. For the BR4γ measurement, 5×1011 events were accumulated over a measurement period of 60 days, which resulted in low statistical uncertainties for the coincident counting between detector pairs (less than 1%). Through simplifying assumptions that neglected the background corrections and efficiency normalisations for each of the 2γ and 4γ decays, a first order approximation of BR4γ was determined as the ratio between measured 4γ events (N4γ) and measured 2γ events (N2γ), such that BR4γ ∼ N4γ N2γ = 4.8 (19) × 10−7. This measured value of BR4γ differs from previous measurements and accepted literature values by a factor of 3."],"dc:identifier.uri":["http://hdl.handle.net/11427/36466"],"dc:publisher.department":["Department of Physics"],"dc:subject":["Physics"],"dc:title":["Multi-photon decay mode spectroscopy of positronium"],"dc:type":["Master Thesis"],"dc:type.qualificationlevel":["Masters","MSc"]},"updated_at":"2026-07-22T22:23:41Z"}