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Showing 1 to 1 of 1 for “"rotation-vibration coupling"”.
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Monte Carlo Methods for the Study of the Ro-Vibrational States of Highly Fluxional Molecules
… application of perturbation theory to the full rotation-vibration Hamiltonian. However, the presence of large amplitude vibrational motions causes the perturbation theory expansion to become slow to converge or even divergent. As a result, the spectra of fluxional systems become difficult to …