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Virginia Tech

Novel polymer architectures: polyrotaxanes

Abstract

dc:description.abstract

Although the synthesis of polymers with highly controlled molecular architectures has gained increased importance due to the rising demand for specialty polymers that possess novel properties, their physical characteristics are direct consequences of the size and constitution of the covalent structures of the polymer. Our program aims to prepare and characterize polymers, whose structures and properties are determined by non-covalent interactions. These novel polymer architectures are comprised of macrocycles threaded by linear macromolecules and are called polyrotaxanes. Polyrotaxanes are considered to be physical analogs of block or graft copolymers or molecular interpenetrating systems. The design and synthesis of the macrocyclic component, "blocking groups" to constrain the macrocycles and the polyrotaxane will be described.

Degree

thesis:*
Name thesis:degree_name
Ph. D.
Level thesis:degree_level
doctoral
Discipline thesis:degree_discipline
Chemistry
Department dc:contributor.department
Chemistry
Grantor dc:publisher
Virginia Tech
Year dc:date.issued
1991

Author and committee

dc:creator, dc:contributor.*
Author dc:creator
  • Engen, Paul Todd
Chairs dc:contributor.committeechair
  • Gibson, Harry W.
  • Riffle, Judy S.
Committee members dc:contributor.committeemember
  • Ward, Thomas C.
  • Wilkes, Garth L.
  • Bell, Harold M.

Rights

dc:rights
Statement dc:rights
  • In Copyright
Language dc:language.iso
en

Identifiers

dc:identifier.*
Dc Identifier Other
etd-07282008-134515
OAI identifier oai:identifier
oai:vtechworks.lib.vt.edu:10919/38882

Chain of custody

source
Harvested from
Virginia Tech
Base URL
vtechworks.lib.vt.edu/oai/request
Last updated
2026-07-22
Source record
OAI-PMH GetRecord
related terms
citation

Engen, Paul Todd. Novel polymer architectures: polyrotaxanes. doctoral thesis, Virginia Tech, 1991. http://hdl.handle.net/10919/38882