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University of Illinois at Urbana-Champaign

The Design of Cyanometallate Cages for Alkali Ion Separation

Abstract

dc:description

The metal sulfide cluster, [(cymene)2Ru3S 2(NCMe)3]2+, reacts with various equivalents of sulfide to give rise to cluster-of-clusters i.e. [(cymene)4Ru 5S4]2+ and [(cymene)6Ru9S 8]2+. The new valence isomer of the [(cymene)4Ru 4S3]2+ was characterized and shown to convert to the black Roussin motif. Finally, this work also demonstrates the potential utility of Ru-S clusters as catalysts for hydrogen production.

Degree

thesis:*
Name thesis:degree_name
Ph.D.
Level thesis:degree_level
Dissertation
Discipline thesis:degree_discipline
Chemistry
Grantor
University of Illinois at Urbana-Champaign
Year dc:date
2015

Author and committee

dc:creator, dc:contributor.*
Author dc:creator
  • Kuhlman, Matthew Lee
Contributors dc:contributor
  • Rauchfuss, Thomas B.

Subjects

dc:subject × 1

Rights

Language dc:language
eng

Identifiers

dc:identifier.*
Identifier
(MiAaPQ)AAI3160908
OAI identifier oai:identifier
oai:www.ideals.illinois.edu:2142/84168

Chain of custody

source
Harvested from
University of Illinois - Urbana-Champaign
Base URL
www.ideals.illinois.edu/oai-pmh
Last updated
2026-07-22
Source record
OAI-PMH GetRecord
citation

Kuhlman, Matthew Lee. The Design of Cyanometallate Cages for Alkali Ion Separation. Dissertation thesis, University of Illinois at Urbana-Champaign, 2015. http://hdl.handle.net/2142/84168