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Purdue University

Hydrogen Loading System Development and Evaluation of Tritiated Substrates to Optimize Performance in Tritium Based Betavoltaics

Abstract

dc:description.abstract

<p>State-of-the-art hydrogen loading system onto thin metallic films based on differential pressure in calibrated chambers has been developed for conditions pressures and temperatures up to 69 bar and 500°C, respectively. Experiments on hydrogen loading on to palladium films of thickness 50 and 250 nm were conducted at pressure ranging from 0.2 bar to 10 bar at temperature 310°C. For first time film hydrogen loading was carried out at 1 bar and at room temperature which temperature. Beta flux exiting surface of metal tritide films has been modeled with MC-SET (Monte Carlo Simulation of Electron Trajectories in solids). Surface beta flux simulations have been improved to account for density changes from tritium loading and decay. Simulation results indicate a 300 nm slab of MgT<sub>2</sub> has a surface flux three times higher than in ScT<sub>2</sub>, and six times higher than in TiT<sub>2</sub>. Commercial betavoltaic cells were tested at different temperature environment for their evaluation and characterization.</p>

Degree

thesis:*
Name thesis:degree_name
Doctor of Philosophy (PhD)
Level thesis:degree_level
Dissertation
Discipline thesis:degree_discipline
Nuclear Engineering
Year
2014

Author and committee

dc:creator, dc:contributor.*
Author dc:creator
  • Adams, Thomas E
Contributors dc:contributor
  • Shripad T. Revankar
  • Dr. Shripad T. Revankar
  • Dr. Audeen Fentiman
  • Dr. Anter El-Azab
  • Dr. Peter Cabauy
  • Dr. Scott Greenway

Subjects

dc:subject × 7

Identifiers

dc:identifier.*
OAI identifier oai:identifier
oai:docs.lib.purdue.edu:open_access_dissertations-1225

Chain of custody

source
Harvested from
Purdue University
Base URL
docs.lib.purdue.edu/do/oai/
Last updated
2026-07-24
Source record
OAI-PMH GetRecord
citation

Adams, Thomas E. Hydrogen Loading System Development and Evaluation of Tritiated Substrates to Optimize Performance in Tritium Based Betavoltaics. Dissertation thesis, 2014. https://docs.lib.purdue.edu/open_access_dissertations/408